Comparison of alternative extraction methods for determining particulate metal fractionation in carbonate-rich Mediterranean soils
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Abstract This review focuses on the concentrations of ionic species (Cl−, NO− 3, SO2− 4, Na+, NH+ 4, K+, Mg2+, and Ca2+) in ambient air in Asian countries during the years 1995–2009. The main likely source of the ionic species Cl−was the ocean while the source of NO− 3and SO2− 4was fossil fuel power stations, and that of Ca2+was terrestrial dust and alkaline particles from cement factory plants. The highest average concentrations of the ionic species Na+and Mg2+in total suspended particulates (TSP) were found in Hong Kong. The highest average concentrations of ionic species Na+, K+, and Ca2+in PM2.5 were found in Nanjing, China, while those of NO− 3and SO2− 4were found in Sha-Lu, Taiwan. The highest average concentrations of Cl−and NH+ 4were found in Beijing, China, while that of Mg2+was found in Shanghai, China. Keywords: ionsparticulatesPM2.5PM10total suspended particulates (TSP)Asian countries Acknowledgement The authors gratefully acknowledge the National Science Council of the ROC (Taiwan) for financial support under project No. NSC 99-2221-E-241-006-MY3
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Urban air quality is continuing to deteriorate. If we want to do something about this problem, we need to know the cause of the pollution. The big problem, not only in Europe, is the high concentrations of particulate matter (PM) in the urban environment. The origin of these particles can be different, including combustion, transport, industry, natural resources, etc. Particulate matter includes a large amount of the finest PM fractions, which can remain in the air for a long time, easily enter respiratory tracks, and damage human health. Particulate matter is also produced by the abrasion of different parts of roads and vehicle fleets and from resuspension road dust, which concerns matter with larger aerodynamic diameters. For this reason, we carried out a series of measurements at various measuring stations in Žilina, Slovakia, during different measuring seasons. The main objective was to find out the diversity of particulate matter sources in Žilina. The search for the particulate matter origin was carried out by particulate matter measurements, determination of the particulate matter fraction concentrations (PM10, PM2.5, and PM1), an investigation on the effect of secondary factors on the particulate matter concentrations, chemical analyses, and multivariate statistical analyses. Varied behavior of the particulate matter with respect to the measurement station and the measurement season was found. Differences in the concentrations of investigated chemical elements contained in the PM were found. Significant changes in the concentrations of particulate matter are caused not only by primary sources (e.g., road traffic in the city of Žilina), but mainly by the negative events (combination of air pollution sources and meteorological conditions). Maximum concentrations of particulate matter PM10 were measured during the winter season at the measuring station on Komenského Street: PM10 126.2 µg/m3, PM2.5 97.7 µg/m3, and PM1 90.4 µg/m3 were obtained using the gravimetric method. The coarse fraction PM2.5-10 was mainly represented by the chemical elements Mg, Al, Si, Ca, Cr, Fe, and Ba, and the fine fraction PM2.5 was represented by the chemical elements K, S, Cd, Pb, Ni, and Zn. Road transport as a dominant source of PM10 was identified from all measurements in the city of Žilina by using the multivariate statistical methods of principal component analysis (PCA) and factor analysis (FA).
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This study attempted to reanalyze the emission property of particulate matter and set up the strategy on the emission reduction of particulate matter by considering the condensable particulate matter additionally as the total particulate matter together with filterable particulate matter. For this, total suspended particles and particulate matter 2.5 emitted in 2013 were selected as pollutants. Fuel classifications were divided into major and minor categories, and the sources were divided into major, medium, and minor categories. Three provinces were set as administrative areas: Gyeonggi-do, Chungcheongnam-do, and Jeollanam-do. The condensable particulate matter emission factors used were obtained from National Institute of Environmental Research. The condensable particulate matter emission factors of liquefied natural gas, diesel, and bunker C oil were measured in boilers with no preventive facilities, and the coal power plant emission factor was obtained at the end of the prevention facility. The condensable particulate matter emissions were calculated by multiplying the particulate matter 2.5 filterable particulate matter emissions by the ratio of the condensable particulate matter emissions to the filterable particulate matter of the National Institute of Environmental Research data. Different patterns of emission sources were observed for each province depending on the consideration of condensable particulate matters. Considering only the filterable particulate matters, the proportion of mobile pollutants was high. On the other hand, considering the condensable particulate matters, the contribution of the nonindustrial combustion category emissions using gaseous fuels, such as city gas, increased in the metropolitan area, whereas the contributions of the manufacturing combustion category emissions increased in the nonmetropolitan areas. Therefore, in the case of collecting energy facilities and the manufacturing burning facilities planned in the local cities in Korea, it is necessary to consider the filterable particulate matter, and condensable particulate matter emission amount.
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