P. E. Barbone

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C. A. Smith

University of Melbourne

A. Torabi

RTX (United States)

A. R. Ravishankara

Colorado State University

P. H. Wine

Georgia Institute of Technology

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Georgia Tech Research Institute

Georgia Institute of Technology

National Oceanic and Atmospheric Administration

University of Melbourne

University of Manchester

INSEAD

Australian National University

PPG Industries (United States)

University of Southern Mississippi

University of Westminster

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N₂O₅ photolysis: Quantum yields for NO₃ and O(³P)

Journal of Geophysical Research Atmospheres (1986)

A. R. Ravishankara P. H. Wine C. A. Smith P. E. Barbone A. Torabi

The quantum yield for the production of NO 3 in the N 2 O 5 photolysis at 248 nm was measured to be unity. The concentration of NO 3 produced upon photolysis was measured using 662‐nm laser absorption. The quantum yields for O( 3 P ) production in the photolysis of N 2 O 5 at 248 nm, 266 nm, 287 nm, and 289 nm were also measured using resonance fluorescence detection of O( 3 P ). The quantum yield for O( 3 P ) decreased from 0.7 at 248 nm to 0.15 at 289 nm. It is postulated that N 2 O 5 photolysis at wavelengths less than 298 nm yields NO 3 + NO + O( 3 P )in addition to NO 3 + NO 2 .

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10.1029/jd091id05p05355

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