Sedimentary rocks and modern sediments sample large volumes of the Earth’s crust, and preserve units that vary greatly in age and composition. Determining the provenance of component minerals is complicated by the ability of some minerals to be recycled through multiple sedimentary cycles, so minerals from completely unrelated sources may end up in the same sedimentary basin. To untangle these multi-stage signals, two or more chemical signatures measured in minerals with different stability are required. For instance, labile minerals, such as feldspar, can break down rapidly during sedimentary transport, while refractory minerals, such as zircon, can be much more resilient and survive repeated recycling. One sedimentary succession suitable for testing this hypothesis is the Upper Carboniferous Millstone Grit Group, a fluvio-deltaic, upward-coarsening sequence of mudstones, sandstones and conglomerates deposited in the Pennine Basin of northern England over c. 14 myr. New isotopic data have been measured in detrital K-feldspar and zircon from five of the seven stages, complementing previous work in the area [1,2,3]. Two K-feldspar Pb isotope peaks at 206Pb/204Pb = 12.5–15.5 and c. 18.4 indicate derivation from Archaean–Proterozoic basement and Caledonian granites, respectively. Zircon U–Pb age peaks at c. 2700, 1000–2000 and 430 Ma reflect a mixture of Archaean basement, Proterozoic sediments and Caledonian granites, while Hf model ages form two broad peaks at c. 4500–3000 and 2300–1500 Ma, indicating contributions from both juvenile and reworked crust. Strong similarities between potential sources in this complicated region mean no one mineral or isotopic system can provide a unique provenance determination. Instead, comparing first-cycle and multi-cycle minerals with different hydrodynamic properties is necessary to untangle the full story. Combining these results with published garnet, monazite and muscovite data demonstrates the power of multi-proxy provenance work, indicating a primary source area in the Greenland Caledonides, with minor contributions from Norway and Scot-land. Comparisons between zircon U–Pb distributions in Palaeozoic sediments suggest long-lived sedimentary systems recycled material around the North Atlantic over c. 100 myr, much of it ultimately derived along the Grenvillian margin of Laurentia. This consistency is interrupted only by regular variations in palaeoflow direction, reflecting tectonic evolution in the region.
Abstract Quartz‐rich sandstones can be produced through multiple sedimentary processes, potentially acting in combination, such as extensive sedimentary recycling or intense chemical weathering. Determining the provenance of such sedimentary rocks can be challenging due to low amounts of accessory minerals, the fact that the primary mineralogy may have been altered during transport, storage or burial and difficulties in the recognition of polycyclic components. This study uses zircon and apatite U‐Pb geochronology, apatite trace elements, zircon‐tourmaline‐rutile indices and petrographic observations to investigate the sedimentary history of mineralogically mature mid‐Carboniferous sandstones of the Tullig Cyclothem, Clare Basin, western Ireland. The provenance data show that the sandstones have been dominantly and ultimately sourced from three basement terranes: older Laurentian‐ associated rocks (ca. 900–2500 Ma) which lay to the north of the basin, peri‐Gondwanan terranes (ca. 500–700 Ma) to the south and igneous intrusive rocks associated with the Caledonian Orogenic Cycle (ca. 380–500 Ma). However, the multi‐proxy approach also helps constrain the sedimentary history and suggests that not all grain populations were derived directly from their original source. Grains with a Laurentian or a Caledonian affinity have likely been recycled through Devonian basins to the south. Grains with a peri‐Gondwanan affinity appear to be first cycle and are potentially derived from south/southwest of the basin. Taken as a whole, these data are consistent with input into the basin from the south and southwest, with the reworking of older sedimentary rocks, rather than intensive first‐cycle chemical weathering, likely explaining the compositional maturity of the sandstones. This study highlights the need for a multi‐proxy provenance approach to constrain sedimentary recycling, particularly in compositionally mature sandstones, as the use of zircon geochronology alone would have led to erroneous provenance interpretations. Zircon, together with U‐Pb geochronology from more labile phases such as apatite, can help distinguish first‐cycle versus polycyclic detritus.
The results of an integrated sedimentological and seismic stratigraphical analysis of three borehole sites on the eastern flank of the Rockall Basin, offshore western Ireland are reported. Two sites were drilled on the western slope of the Porcupine High, above the North and South Bróna basins (boreholes 83/20-sb01, 83/24-sb01 and 83/24-sb02), and one on the northern flank of the Porcupine High (16/28-sb01), above the Macdara Basin. The cores establish that the half-graben basins marginal to the eastern Rockall Basin contain Jurassic deposits and that they were inverted sometime in the Late Jurassic or Early Cretaceous. An angular unconformity above the Bróna basins is overlain by a condensed, tripartite Cretaceous succession (‘brownsand’, ‘greensand’, chalky micrite) that records stepwise deepening, with evidence for a Cenomanian-Turonian phase of normal faulting. Above the Macdara Basin, the unconformity is overlain by a basalt that was cored at the 16/28 site and is interpreted to represent a flow of Cretaceous age derived from the Drol Igneous Centre. At all three borehole sites, Cretaceous strata are onlapped (or downlapped) by Paleocene-Eocene strata that display evidence of a minor episode of fault reactivation above the Bróna basins. Cored Eocene strata vary from clastic to carbonate-prone from north to south and smectitic clays are common at the 16/28 site. Post-Mid-Eocene westward tilting of the Rockall slope rotated the Eocene stratigraphy and the underlying Cretaceous deposits (including the lava flow in the 16/28 area) at least 3° down to the west. Slope development resulted in extensional sliding and the erosion of the C30 deep-water unconformity that is onlapped by Miocene slope deposits. C30 was cored in the 83/20 area where it cuts down into Cretaceous strata and is crusted with phosphates and the Cretaceous beneath Mn-impregnated.