Baobin Wang

Shandong Academy of Sciences

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Jiachuan Chen

Qilu University of Technology

Guihua Yang

Qilu University of Technology

Chenglong Qiu

Shandong Academy of Sciences

Kai Zhang

Qilu University of Technology

Penghua Zhao

Shaanxi Provincial People's Hospital

Lei Dai

Jiangnan University

Lucian A. Lucia

North Carolina State University

Yonghao Ni

University of New Brunswick

Jiaming Fan

Chongqing Medical University

Jinze Li

Dongbei University of Finance and Economics

Cooperative Institutions

Qilu University of Technology

Shandong Academy of Sciences

University of New Brunswick

Shaanxi University of Science and Technology

North Carolina State University

Tianjin University

Chinese Academy of Sciences

Dalian University of Technology

Harbin Institute of Technology

Nanjing University of Science and Technology

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One-pot furfural production from sustainable biomass-derived sugars using a functionalized covalent organic framework as a heterogeneous catalyst

Green Chemistry (2024)

Peng Gan Kai Zhang Zhihao Li Chengxiang Zhang Guihua Yang

This paper presents an innovative study on the green production of furfural using a covalent organic framework as a heterogeneous catalyst, thereby achieving efficient furfural production from sustainable biomass-derived sugars.

5-hydroxymethylfurfural

10.1039/d4gc00643g

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Citations (3)

Highly Active N, S Codoped Porous Carbon Derived from Lignin-Rich Pulping Waste Liquor for Supercapacitors and Oxygen Reduction Reaction

Energy & Fuels (2024)

Penghua Zhao Jiachuan Chen Lei Zhang Chenglong Qiu Baobin Wang

Heteroatom-doped porous carbon has become a key material in the field of supercapacitors (SCs) and the oxygen reduction reaction (ORR). Here, eucalyptus pulping red liquor was used as the starting material for a straightforward one-step NH4Cl-assisted carbonization technique that produced a nitrogen and sulfur codoped bifunctional porous carbon material. The sulfur in sodium lignosulfonate was used as a S atom dopant. NH4Cl added to the red liquor can not only produce NaCl as a template but also as a nitrogen source. The resulting carbons possess rich hierarchical porous structures and high specific surface area (1092 m2 g–1) and ID/IG ratio (1.04), leading to remarkable electrocatalytic activity with a specific capacitance of 326 F g–1 at 0.5 A g–1 for capacitance and an identical onset and half-wave potentials of 0.988 V vs reversible hydrogen electrode (RHE) and 0.847 V vs RHE for the ORR, as compared with the benchmark Pt/C catalyst. Furthermore, when BLC-N/S-1000 was used as an electrocatalyst in an air electrode of a zinc–air battery, it showed superior long-term stability for 356 h at 5 mA cm–2 and 20 min/cycle. Results in the present work pave a new green method to convert abundant low-cost biomass into high-end heteroatom-doped carbons with rich hierarchical porous structures for electrochemical energy devices.

Heteroatom

Carbon fibers

10.1021/acs.energyfuels.3c03915

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Citations (5)

A self-assembling guar gum hydrogel for efficient oil/water separation in harsh environments

Separation and Purification Technology (2019)

Lei Dai Ting Cheng Yan Wang Baobin Wang Chao Duan

Sodium periodate

Guar gum

Biofouling

10.1016/j.seppur.2019.05.070

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Citations (37)

High performance bio-supercapacitor electrodes composed of graphitized hemicellulose porous carbon spheres

Frontiers in Bioengineering and Biotechnology (2022)

Zhili Zhang Fengfeng Li Jiachuan Chen Guihua Yang Xingxiang Ji

A template-free and one-step carbonization process was developed for fabricating graphitic porous carbon spheres (GPCSs) on hemicelluloses as the electrode material for supercapacitors. This method is green, low-energy, and less time consuming compared to the conventional two-step process (pore-forming and graphitizing). It uses K2FeO4, a mild activating agent that fulfills synchronous activation and graphitization. The GPCSs is regular spherical shape, have high nanoporosity, a large specific surface area (1,250 m2 g-1), and have a high graphitization degree. A unique structural advantage includes a rich interconnected conductive network for electron transfer that shortens the ion transport distance of the electrolyte. Remarkably, the GPCSs electrode displays outstanding electrochemical performance including high specific capacitance (262 F g-1 at 1.0 A g-1), rate capability energy (80%, 20 A g-1), and excellent cycling stability (95%, 10,000 cycles). This work represents a powerful methodology to develop sustainable and low-cost energy storage devices from hemicellulose.

Hemicellulose

Carbon fibers

10.3389/fbioe.2022.1030944

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Citations (3)

Wood-derived Fe cluster-reinforced asymmetric single-atom catalysts and weather-resistant organohydrogel for wide-temperature flexible Zn–air batteries

Energy & Environmental Science (2024)

Jiachuan Chen Chenglong Qiu Lei Zhang Baobin Wang Penghua Zhao

All wood-based wide-temperature flexible Zn–air battery.

10.1039/d4ee01226g

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Citations (16)

Multifunctional self-assembling hydrogel from guar gum

Chemical Engineering Journal (2017)

Lei Dai Liqiang Zhang Baobin Wang Bo Yang I. B. Khan

Guar gum

Sodium periodate

Periodate

Vicinal

10.1016/j.cej.2017.08.041

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Citations (80)

From wood to flexible Zn-air Battery: Fe3O4 nanoparticles synergistic single iron atoms on N-doped carbon nanosheets electrocatalyst and Lignosulfonate-Functionalized gel electrolyte

Chemical Engineering Journal (2024)

Penghua Zhao Lei Zhang Jiachuan Chen Chenglong Qiu Baobin Wang

Polyvinyl Alcohol

Carbon fibers

10.1016/j.cej.2024.149415

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Citations (7)

Hydrothermal Carbonization of Corncob Residues for Hydrochar Production

Energy & Fuels (2014)

Lei Zhang Qiang Wang Baobin Wang Guihua Yang Lucian A. Lucia

Upgrading corncob residues (CCR) to a high quality energy resource is an effective utilization of an underutilized industrial lignocellulose waste. A hydrothermal carbonization technique was therefore employed to generate a high heating value (HHV) hydrochar. Results showed that its HHV increased 47% after treatment at 230 °C for 1.5 h. Decreases in H/C and O/C verified that reductions in C and O reactions were occurring following hydrothermal carbonization. The chemical and thermal properties of the final hydrochar as analyzed by FT-IR, TG/DTG, and XRD analyses indicated that dehydration and decarboxylation were the predominant pathways for the C and O reductions. The present hydrothermal carbonization process is offered as a promising approach to upgrade CCR to a high heating value hydrochar under mild conditions.

Hydrothermal Carbonization

Corncob

Heat of combustion

10.1021/ef502462p

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Citations (169)